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Wingenfelder, U., Hansen, C., Furrer, G., & Schulin, R. (2005). Removal of heavy metals from mine waters by natural zeolites. Environ Sci Technol, ES & T, 39(12), 4606–4613.
Keywords: Groundwater problems and environmental effects Pollution and waste management non radioactive remediation heavy metal mine drainage acid mine drainage; acidification; Central Europe; chemical composition; chemical fractionation; dissolved materials; Europe; framework silicates; geochemistry; grain size; heavy metals; hydrochemistry; ion exchange; lead; metals; mines; mining; mobilization; models; pH; pollutants; pollution; precipitation; remediation; samples; silicates; spectra; Switzerland; toxic materials; X-ray diffraction data; X-ray fluorescence spectra; zeolite group
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Hulshof, A. H. M., Blowes, D. W., & Douglas Gould, W. (2006). Evaluation of in situ layers for treatment of acid mine drainage: A field comparison. Water Res, 40(9), 1816–1826.
Abstract: Reactive treatment layers, containing labile organic carbon, were evaluated to determine their ability to promote sulfate reduction and metal sulfide precipitation within a tailings impoundment, thereby treating tailings effluent prior to discharge. Organic carbon materials, including woodchips and pulp waste, were mixed with the upper meter of tailings in two separate test cells, a third control cell contained only tailings. In the woodchip cell sulfate reduction rates were 500 mg L-1 a-1, (5.2 mmol L-1 a-1) this was coupled with the gradual removal of 350 mg L-1 Zn (5.4 mmol L-1). Decreased δ13CDIC values from -3‰ to as low as -12‰ indicated that sulfate reduction was coupled with organic carbon oxidation. In the pulp waste cell the most dramatic change was observed near the interface between the pulp waste amended tailings and the underlying undisturbed tailings. Sulfate reduction rates were 5000 mg L-1 a-1 (52 mmol L-1 a-1), Fe concentrations decreased by 80–99.5% (148 mmol L-1) and Zn was consistently <5 mg L-1. Rates of sulfate reduction and metal removal decreased as the pore water migrated upward into the shallower tailings. Increased rates of sulfate reduction in the pulp waste cell were consistent with decreased δ13CDIC values, to as low as -22‰, and increased populations of sulfate reducing bacteria. Lower concentrations of the nutrients, phosphorus, organic carbon and nitrogen in the woodchip material contribute to the lower sulfate reduction rates observed in the woodchip cell.
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Reisinger, R. W., & Gusek, J. (1999). Mitigation of water contamination at the historic Ferris-Haggarty Mine, Wyoming. Min. Eng., 51(8), 49–53.
Abstract: An historic underground copper mine in Wyoming is discharging neutral but copper-laden water into a pristine creek. The EPA-deferred site qualifies for reclamation by the Wyoming Abandoned Mine Land (AML) program. The cleanup goal is to restore the discharge so that the creek can eventually support a trout fishery. Hydrological and geochemical investigations underground have suggested two sources of mine water: one clean and the other containing copper. Results of bench- and pilot-scale tests support the viability of using low-cost passive treatment techniques to reduce copper concentrations in the near-freezing mine discharge.
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Dunn, J., Russell, C., & Morrissey, A. (1999). Remediating historic mine sites in Colorado. Min. Eng., 51(8), 32–35.
Abstract: This article provides examples of reclamation and remediation in Colorado watersheds. The projects were undertaken by the US Environmental Protection Agency (EPA) Region 8, in cooperation with the Colorado Division of Minerals and Geology (CDMG), Colorado Department of Public Health and Environment (CDPHE), US Forest Service (USFS), the Bureau of Land Management (BLM), Bureau of Reclamation (BOR) and the US Geological Survey (USGS). These agencies collaborated on the environmental problems at abandoned mines. These samples involved the interaction of surface and ground waters with sulfide-bearing rocks, mine workings and surface mine spoils that produce acid solutions charged with heavy metals that are toxic to organisms. In these examples, acid mine drainage from historic mines in Colorado has been approached cooperatively with stakeholders. Each example emphasizes one aspect of the three-stage process. These stages include characterization and prioritization, hydrologic controls and the evaluation of long-term remediation activities.
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Eger, P., Melchert, G., & Wagner, J. (2000). Using passive treatment systems for mine closure – A good approach or a risky alternative? Min. Eng., 52(9), 78–83.
Abstract: In 1991, LTV Steel Mining decided to close an open-pit taconite mine in northeastern Minnesota using a passive-treatment approach consisting of limiting infiltration into the stockpiles and wetland treatment to remove metals. More than 50 Mt (55 million st) of sulfide-containing waste had been stockpiled adjacent to the mine during its 30 years of operation. Drainage from the stockpiles contained elevated levels of copper, nickel, cobalt and zinc. Nickel is the major trace metal in the drainages. Before the closure, the annual median concentrations ranged from 1.5 to 50 mg/L. Copper, cobalt and zinc are also present but they are generally less than 5% of the nickel values. Median pH levels range from 5 to 7.5, but most of the stockpile drainages have pH levels greater than 6.5. Based on the chemical composition of each stockpile, a cover material was selected. The higher the potential that a stockpile had to produce acid drainage, the lower the permeability of the capping material required. Covers ranged from overburden soil removed at the mine to a flexible plastic liner. Predictions of the reduction in infiltration ranged from 40% for the native soil to more than 90% for the plastic liner. Five constructed wetlands have been installed since 1992. They have removed 60% to 90% of the nickel in the drainages. Total capital costs for all the infiltration reduction and wetlands exceeded $6.5 million, but maintenance costs are less than 1% of those for an active treatment plant. Because mine-drainage problems can continue for more than 100 years, the lower annual operating costs should pay for the construction of the wetland-treatment systems within seven years.
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