| Records |
| Author |
Foucher, S.; Battaglia-Brunet, F.; Ignatiadis, I.; Morin, D. |
| Title |
Treatment by sulfate-reducing bacteria of Chessy acid-mine drainage and metals recovery |
Type |
Journal Article |
| Year |
2001 |
Publication |
Chemical Engineering Science |
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| Volume |
56 |
Issue |
4 |
Pages |
1639-1645 |
| Keywords |
Acid mine drainage Sulfate-reducing bacteria Sulfide precipitation Hydrogen transfer Fixed bed column reactor |
| Abstract |
Acid-mine drainage can contain high concentrations of heavy metals and release of these contaminants into the environment is generally avoided by lime neutralization. However, this classical treatment is expensive and generates large amounts of residual sludge. The selective precipitation of metals using H2S produced biologically by sulfate-reducing bacteria has been proposed as an alternative process. Here, we report on experiments using real effluent from the disused Chessy-les-Mines mine-site at the laboratory pilot scale. A fixed-bed bioreactor, fed with an H2/CO2 mixture, was used in conjunction with a gas stripping column. The maximum rate of hydrogen transfer in the bioreactor was determined before inoculation. kLa was deduced from measurements of O2 using Higbie and Danckwert's models which predict a dependence on diffusivity. The dynamic method of physical absorption and desorption was used. The maximum rate of H2 transfer suggests that this step should not be a limiting factor. However, an increase in H2 flow rate was observed to induce an increase in sulfate reduction rate. For the precipitation step, the gas mixture from the bioreactor was bubbled into a stirred reactor fed with the real effluent. Cu and Zn could be selectively recovered at pH=2.8 and pH=3.5, respectively. Other impurities such as Ni and Fe could also be removed at pH=6 by sulfide precipitation. Part of the outlet stream from the bioreactor was used to regulate and maintain the pH during sulfide precipitation by feeding the outlet stream back into the bioreactor. The replacement of synthetic medium with real effluent had a positive effect on sulfate reduction rate which increased by 30-40%. This improvement in bacterial efficiency may be related to the large range of oligo-elements provided by the mine-water. The maximum sulfate reduction rate observed with the real effluent was 200 mgl-1 h-1, corresponding to a residence time of 0.9 day. A preliminary cost estimation based on a treatment rate of 5 m3 h-1 of a mine effluent containing 5 gl-1 SO42- is presented. |
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0009-2509 |
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Feb.; Treatment by sulfate-reducing bacteria of Chessy acid-mine drainage and metals recovery; file:///C:/Dokumente%20und%20Einstellungen/Stefan/Eigene%20Dateien/Artikel/10064.pdf; Science Direct |
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CBU @ c.wolke @ 10064 |
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54 |
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| Author |
Banks, S.B.; Banks, D. |
| Title |
Abandoned mines drainage; impact assessment and mitigation of discharges from coal mines in the UK |
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Book Chapter |
| Year |
2001 |
Publication |
Geoenvironmental engineering Engineering Geology |
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Issue |
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Pages |
31-37 |
| Keywords |
abandoned mines coal mines cost discharge drainage England environmental effects Europe feasibility studies Great Britain mine drainage mines mitigation pollution remediation Scotland United Kingdom Western Europe 22, Environmental geology |
| Abstract |
The UK has a legacy of pollution caused by discharges from abandoned coal mines, with the potential for further pollution by new discharges as groundwaters continue to rebound to their natural levels. In 1995, the Coal Authority initiated a scoping study of 30 gravity discharges from abandoned coal mines in England and Scotland. Mining information, geological information and water quality data were collated and interpreted in order to allow a preliminary assessment of the source and nature of each of the discharges. An assessment of the potential for remediation was made on the basis of the feasibility and relative costs of alternative remediation measures. Environmental impacts of the discharges and of the proposed remediation schemes were also assessed. The results, together with previous Coal Authority studies of discharges in Wales, were used by the Coal Authority, in collaboration with the former National Rivers Authority and the former Forth and Clyde River Purification Boards, to rank discharge sites in order of priority for remediation. |
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60 |
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Yong, R.N.; Thomas, H.R. |
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Abandoned mines drainage; impact assessment and mitigation of discharges from coal mines in the UK; GeoRef; English; 2001-052748; British Geotechnical Society, second conference on Geoenvironmental engineering, London, United Kingdom, Sept. 1999 References: 12; illus. incl. 2 tables |
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CBU @ c.wolke @ 16515 |
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31 |
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| Author |
Ye, Z.H. |
| Title |
Removal and distribution of iron, manganese, cobalt, and nickel within a Pennsylvania constructed wetland treating coal combustion by-product leachate |
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Journal Article |
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2001 |
Publication |
Journal of Environmental Quality |
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30 |
Issue |
4 |
Pages |
1464-1473 |
| Keywords |
mine water treatment |
| Abstract |
A flow-through wetland treatment system was constructed to treat coal combustion by-product leachate from an electrical power station at Springdale, Pennsylvania. In a nine-compartment treatment system, four cattail (Typha latifolia L.) wetland cells (designated Cells I through 4) successfully removed iron (Fe) and manganese (Mn) from the inlet water; Fe and Mn concentrations were decreased by an average of 91% in the first year (May 1996-May 1997), and by 94 and 98% in the second year (July 1997-June 1998), respectively. Cobalt (Co) and nickel (Ni) were decreased by an average of 39 and 47% in the first year, and 98 and 63% in the second year, respectively. Most of the metal removed by the wetland cells was accumulated in sediments, which constituted the largest sink. Except for Fe, metal concentrations in the sediments tended to be greater in the top 5 em of sediment than in the 5- to 10- or 10- to 15-cm layers, and in Cell I than in Cells 2, 3, and 4. Plants constituted a much smaller sink for metals; only 0.91, 4.18, 0.19, and 0.38% of the Fe, Mn, Co, and Ni were accumulated annually in the aboveground tissues of cattail, respectively. A greater proportion of each metal (except Mn) was accumulated in cattail fallen litter and submerged Chara (a macroalga) tissues, that is, 2.81, 2.75, and 1.05% for Fe, Co, and Ni, respectively. Considerably higher concentrations of metals were associated with cattail roots than shoots, although Mn was a notable exception. |
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Removal and distribution of iron, manganese, cobalt, and nickel within a Pennsylvania constructed wetland treating coal combustion by-product leachate; Wos:000174863000040; Times Cited: 15; ISI Web of Science |
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CBU @ c.wolke @ 17061 |
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122 |
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| Author |
Chung, I.J. |
| Title |
Immobilization of arsenic in tailing by using iron and hydrogen peroxide |
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Journal Article |
| Year |
2001 |
Publication |
Environ. Technol. |
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| Volume |
22 |
Issue |
7 |
Pages |
831-835 |
| Keywords |
mine water treatment |
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Under environmental conditions, arsenic (As) reveals anionic behavior and is converted into various forms in accordance with the Eh/pH condition. This causes the difficulty of treating As with other heavy metals in tailing. This study was carried out to develop the immobilization method of arsenic in tailing as ferric arsenate (FeAsO4) using hydrogen peroxide. According to experimental results, the extracted concentrations of arsenic and iron (Fe) from tailing were reduced up to 84% and 93%, respectively. In the experiment using pure Pyrite (FeS2) and As solution, As concentration decreased with an increase of hydrogen peroxide dosage. The experimental results of re-extraction showed that only 10% of As and 20% of Fe were extracted in the case of using hydrogen peroxide. As a result, the long-term stability of this method was clarified. |
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Immobilization of arsenic in tailing by using iron and hydrogen peroxide; Wos:000170195000008; Times Cited: 0; ISI Web of Science |
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CBU @ c.wolke @ 17046 |
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123 |
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| Author |
Goulet, R.R. |
| Title |
Changes in dissolved and total Fe and Mn in a young constructed wetland: Implications for retention performance |
Type |
Journal Article |
| Year |
2001 |
Publication |
Ecological Engineering |
Abbreviated Journal |
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| Volume |
17 |
Issue |
4 |
Pages |
373-384 |
| Keywords |
mine water treatment |
| Abstract |
Surface-flow wetlands are generally considered sinks for Fe and Mn but they may also export and affect the partitioning of these metals. This study was undertaken to evaluate the effect of a young constructed wetland on the retention and transformation of both dissolved and particulate Fe and Mn. Duplicate water samples were collected every three days at the inlet and outlet structures of the Monahan Wetland, Kanata, Ontario, from spring of 1997 to 1999. While on a yearly basis the wetland showed significant retention of che dissolved phase, the retention of total Fe and Mn was poor. There were strong seasonal differences in retention and, during the winter, the wetland was a source. The wetland transformed dissolved into particulate Fe and Mn from spring to fall whereas during the winter, dissolved Fe and Mn were released. Changes in pH, alkalinity and temperature could explain 11% and 40% of the outlet variation in the ratio of dissolved to total Fe and Mn respectively. Furthermore, from spring to late summer, planktonic algal biomass was negatively related to the ratio of dissolved to total Fe and Mn implying a role in Fe and Mn transformations in young wetlands where emergent and submerged vegetation have yet to dominate the system. (C) 2001 Elsevier Science B.V. All rights reserved. |
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Changes in dissolved and total Fe and Mn in a young constructed wetland: Implications for retention performance; Wos:000169881900004; Times Cited: 5; ISI Web of Science |
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CBU @ c.wolke @ 17050 |
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124 |
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